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中国腐蚀与防护学报  2019, Vol. 39 Issue (5): 404-410    DOI: 10.11902/1005.4537.2019.174
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机械摩擦磨损与电化学腐蚀在特殊环境中的作用机制
陈嘉晨,王忠维,乔利杰,岩雨()
北京科技大学 新材料技术研究院腐蚀与防护中心 北京材料基因工程高精尖创新中心 北京 100083
Interaction between Friction-wear and Corrosion in Special Environment
CHEN Jiachen,WANG Zhongwei,QIAO Lijie,YAN Yu()
Beijing Advanced Innovation Center for Materials Genome Engineering, Corrosion and Protection Center, Institute of Advanced Materials and Technology, University of Science and Technology Beijing, Beijing 100083, China
全文: PDF(804 KB)   HTML
摘要: 

生物磨蚀是机械摩擦磨损与电化学腐蚀在生物环境中的耦合作用。由于材料或部件的服役环境中存在着生物大分子和细胞组织，因此生物磨蚀比一般的磨蚀机理更加复杂。生物磨蚀影响最明显的两个应用是人工关节植入体和人工牙种植体。本文综述了目前关于磨蚀的研究进展，并着重总结了生物磨蚀机理的研究和生物磨蚀对材料界面和表面的影响。对于磨蚀来说，摩擦磨损与腐蚀的交互作用是研究的核心，这两个分量不能孤立的进行研究。并且对于生物磨蚀、蛋白质的吸附、磨蚀对蛋白质的影响以及摩擦膜的生成机理等，都有待深入系统的研究。本文在对生物磨蚀总结的基础上，提出该领域未来的发展方向和前景。
关键词 ： 摩擦磨损,  腐蚀,  人工关节,  纳米晶,  生物膜    
Abstract：

The interaction of mechanical friction-wear and electrochemical corrosion in biological environments is named as bio-tribocorrosion. Due to large bio molecules in the surrounding environment, the adsorption of such molecules has great influence on the tribocorrosion behaviour of implant materials. In terms of the influence of bio-tribocorrosion, both the artificial joint implants and dental implants encounters obviously issues of bio-tribocorrosion. In this paper, we summarized the current status of research on bio-tribocorrosion with the emphasis on the mechanisms of relevant processes and the effect of bio-tribocorrosion on the surface microstructure of implants. It is noted that to choose proper testing methods is a very important matter for assessing the bio-tribocorrosion process. Besides, the future trend and directions of research in this area are also put forward.
Key words： tribology    corrosion    artificial joint    nanocrystalline    biofilm
收稿日期: 2019-09-29     
ZTFLH:  TQ174  
基金资助:国家自然科学基金(U1660104)
通讯作者: 岩雨     E-mail: yanyu@ustb.edu.cn
Corresponding author: Yu YAN     E-mail: yanyu@ustb.edu.cn
作者简介: 陈嘉晨，男，1995年生，博士生
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陈嘉晨
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引用本文:

陈嘉晨,王忠维,乔利杰,岩雨. 机械摩擦磨损与电化学腐蚀在特殊环境中的作用机制[J]. 中国腐蚀与防护学报, 2019, 39(5): 404-410.
Jiachen CHEN, Zhongwei WANG, Lijie QIAO, Yu YAN. Interaction between Friction-wear and Corrosion in Special Environment. Journal of Chinese Society for Corrosion and protection, 2019, 39(5): 404-410.

链接本文:

https://www.jcscp.org/CN/10.11902/1005.4537.2019.174      或      https://www.jcscp.org/CN/Y2019/V39/I5/404

图1  磨蚀反应中可能与腐蚀发生交互作用的因素
Contact stateRelated reaction
Contact load and form

1. Contact pressure (surface and subsurface) and contact area

2. Elastic or elastic-plastic or complete plastic reactions on surfaces and subsurfaces

3. Surface deformation (elastic or permanent deformation)

Relative motion under loading conditions (causing wear in corrosive environments)

1. Depassivation of passivated surfaces

2. Corrosion potential (mixed potential of wear and non-wear area)

3. Causing phase transition on the surface or near the surface

4. Repassivation kinetics

5. Local mass transfer acceleration

6. Increase in contact temperature

7. Increase in roughness and corresponding area

8. Change of surface composition

9. Formation of a mechanical mixing layer, which may contain debris

10. Wear area and the non-wear area constitute a couple pair

11. Cause surface hardening

12. Affects the shear strength of rough/rough surface joints and causes adhesion

Changing load in dynamic contact

1. Self-corrosion potential

2. Local current density

3. Area of active anode and anode site position[4]

4. Surface recovery time

5. Change the wear mechanism or wear rate

Frictionr- corrosion

1. Effect of friction

2. Local environmental pH

3. Total surface loss (mechanical and electrochemical)

Wear debrisResulting metal abrasives corrode in the environment causing secondary release of ions
表1  腐蚀/表面上的影响因素
图2  钴铬钼合金在小牛关节滑液中的开路电位和摩擦系数随时间的变化曲线
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