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中国腐蚀与防护学报  2021, Vol. 41 Issue (3): 277-288    DOI: 10.11902/1005.4537.2020.089
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非晶合金耐蚀性研究进展
王东亮, 丁华平, 马云飞, 龚攀(), 王新云
华中科技大学材料科学与工程学院 材料成形与模具技术国家重点实验室 武汉 430074
Research Progress on Corrosion Resistance of Metallic Glasses
WANG Dongliang, DING Huaping, MA Yunfei, GONG Pan(), WANG Xinyun
State Key Laboratory of Material Processing and Die & Mould Technology, School of Material Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
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摘要: 

综述了非晶合金耐蚀性的研究现状，归纳了合金成分、合金结构、制备工艺、腐蚀介质、表面状态、加载应力以及其他重要因素对非晶合金耐蚀性的影响规律，总结了非晶合金耐蚀性能的改善途径，并对非晶合金耐蚀性研究方面存在的问题和今后的发展趋势进行了探讨和展望。
关键词 ： 非晶合金,  耐蚀性,  影响因素,  改善方法    
Abstract：

Because of their unique amorphous structure, metallic glasses (MGs) exhibit better corrosion resistance compared with traditional crystalline metals and alloys. Thus, MGs have broad application prospects as novel corrosion-resistant materials. The research progress of corrosion resistance of MGs was summarized. The influence factors, such as the alloy composition, microstructure, preparation method, corrosion environment, surface state, stress state etc. on the corrosion resistance of MGs were introduced. The routes to improve the corrosion resistance of MGs were proposed. Finally, the future development trends of corrosion resistance of MGs were discussed and prospected.
Key words： metallic glass    corrosion resistance    influence factor    improving method
收稿日期: 2020-05-24     
ZTFLH:  TG174  
基金资助:湖北省自然科学基金(2018CFB576);国家自然科学基金(51725504);中央高校基本科研业务费(2018KFYRCPT001)
通讯作者: 龚攀     E-mail: pangong@hust.edu.cn
Corresponding author: GONG Pan     E-mail: pangong@hust.edu.cn
作者简介: 王东亮，男，1997年生，硕士生
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王东亮, 丁华平, 马云飞, 龚攀, 王新云. 非晶合金耐蚀性研究进展[J]. 中国腐蚀与防护学报, 2021, 41(3): 277-288.
Dongliang WANG, Huaping DING, Yunfei MA, Pan GONG, Xinyun WANG. Research Progress on Corrosion Resistance of Metallic Glasses. Journal of Chinese Society for Corrosion and protection, 2021, 41(3): 277-288.

链接本文:

https://www.jcscp.org/CN/10.11902/1005.4537.2020.089      或      https://www.jcscp.org/CN/Y2021/V41/I3/277

图1  非晶合金 (MGs) 和常见不锈钢 (SSs) 在3种溶液中的腐蚀行为
ElementContent x(Atomic fraction / %)Base alloy (Atomic fraction / %)Corroding solutionEffect on corrosion resistanceReferences
Sr0~1%Mg66Zn30Ca4-xSrxPhosphate-buffered salineEnhanced[33]
1%~1.5%Deteriorated
Y0~2.5%(Zr58Nb3Cu16Ni13Al10)100-xYx0.5 mol/L H2SO4Deteriorated[30]
1%(Zr55Al10Cu30Ni5)99YxPhosphate-buffered salineEnhanced[20]
Nb0~20%Zr46Cu(30.14-x)NbxAg8.36Al8Be7.50.1 mol/L HClEnhanced[34]
0.5 mol/L NaClEnhanced
0.5 mol/L H2SO4Enhanced
Nd0~0.5%Mg68-xZn28Ca4NdxSimulated body fluidEnhanced[25]
0.5%~1.5%Deteriorated
Cr0~30%CrxFe56-xCo7Mo14C15B6Y21 mol/L HClEnhanced[32]
30%~45%No difference
0~29.4%CrxFe58.8-xMo14.7C14.7B9.8Y21 mol/L HClEnhanced[35]
29.4%~44.1%No difference
0~8.3%Fe71.4-xC7.1Si4.4B6.5P8.6CrxAl2.09.7 mol/L H2SO4Enhanced[22]
8.3%~12.3%Deteriorated
0~5%Fe79.5-xSi9.5B11Crx0.1 mol/L NaClEnhanced[36]
B0~5%Zr66.7-xNi33.3Bx0.5 mol/L NaClB0.3＞B0.1, B0.5＞B0[19]
1 mol/L HClB0.5＞B0.1, B0.3＞B0
2 mol/L NaOHB0.1＞B0.5＞B0.3, B0
Co0~4%(Zr46Cu46Al8)100-xCox3.5%NaClEnhanced[28]
Ti0~4%(Cu37.6Zr46Ag8.4Al8)100-xTix1 mol/L NaOHEnhanced[26]
1 mol/L H2SO4Enhanced
1 mol/L H2SO4+0.01 mol/L NaClEnhanced
1 mol/L H2SO4+0.1 mol/L NaClEnhanced
Ag0~9%Zr53Co23.5-xAl23.5AgxPhosphate-buffered salineEnhanced[29]
Si0~2%Fe85.2SixB9P5-xCu0.8Boric-borate buffer solutionEnhanced[37]
C0~3%Fe73.5Cu1Nb3Si13.5CxB99-x0.1 mol/L H2SO4Enhanced[38]
Mn0~1.5%(Mg65Zn30Ca5)100-xMnxSimulated body fluidDeteriorated[24]
Ce3%~7%Al93-xCo7Cex0.6 mol/L HClCe4 is the best[39]
Au0~3%Ca47Mg18Zn35-xAuxRinger's solutionEnhanced[40]
P0~15%Fe43Cr16Mo16(C, B, P)251, 6, 12 mol/L HClP＞B, C[21]
Ni0~0.4%[(Fe1-xNix)0.75B0.2Si0.05]96Nb40.5 mol/L HClEnhanced[27]
0.5 mol/L H2SO4Enhanced
0.5 mol/L NaOHEnhanced
Hf0~5%Zr55Ti3HfxCu32-xAl100.6 mol/L NaClEnhanced[31]
1 mol/L HClEnhanced
1 mol/L H2SO4Enhanced
表1  添加合金元素对非晶合金耐蚀性的影响总结
图2  Zr65Cu17.5Fe10Al7.5铸态和等温退火不同时间后在3.5%NaCl溶液中动电位极化曲线[41]
图3  铸态Cu47.5Zr47.5Al5棒 (5 mm) 和退火态棒 (3 mm) 在海水溶液中腐蚀表面的FESEM像[47]
图4  非晶合金Zr50.7Ni28Cu9Al12.3在1 mol/L HCl、0.5 mol/L H2SO4和0.5 mol/L NaCl溶液中Ecorr和pH值的关系[57]
图5  Co-Cr-Mo非晶合金腐蚀试验后注入C和未处理的表面形貌[72]
图6  室温下几种合金在3.5%NaCl溶液中的动电位极化曲线[79]
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