功能性超疏水涂层在极地抗冰领域的应用研究进展

doi:10.11902/1005.4537.2023.046

中国腐蚀与防护学报

2024, Vol. 44

Issue (1): 1-14 CSTR: 32134.14.1005.4537.2023.046 DOI: 10.11902/1005.4537.2023.046

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功能性超疏水涂层在极地抗冰领域的应用研究进展

姜伯晨¹^,², 类延华¹(

), 张玉良¹, 李晓峰¹, 刘涛¹(

), 董丽华¹

^1.上海海事大学海洋科学与工程学院上海 201306
^2.江苏航运职业技术学院智能制造与信息学院南通 226000

Research Progress on Application of Functional Superhydrophobic Coatings for Anti-icing in Polar Regions

JIANG Bochen¹^,², LEI Yanhua¹(

), ZHANG Yuliang¹, LI Xiaofeng¹, LIU Tao¹(

), DONG Lihua¹

^1.College of Ocean Science and Engineering, Shanghai Maritime University, Shanghai 201306, China
^2.School of Intelligent Manufacturing and Information, Jiangsu Shipping College, Nantong 226000, China

引用本文:

姜伯晨, 类延华, 张玉良, 李晓峰, 刘涛, 董丽华. 功能性超疏水涂层在极地抗冰领域的应用研究进展[J]. 中国腐蚀与防护学报, 2024, 44(1): 1-14.
Bochen JIANG, Yanhua LEI, Yuliang ZHANG, Xiaofeng LI, Tao LIU, Lihua DONG. Research Progress on Application of Functional Superhydrophobic Coatings for Anti-icing in Polar Regions[J]. Journal of Chinese Society for Corrosion and protection, 2024, 44(1): 1-14.

全文: PDF(12937 KB) HTML

摘要:

就结冰机理、超疏水表面浸润理论和界面的抗冰特性进行了综述，然后对不同方法制备的超疏水涂层在抗冰领域的应用进行了讨论和总结。最后，针对超疏水涂层在除冰方面存在的缺陷，提出了具有光热、电热等功能性超疏水涂层策略，并全面介绍了目前的研究现状。

关键词 ：抗冰涂层, 超疏水, 光热除冰, 电热除冰, 极地

Abstract：

With the development and utilization of polar routes and rich resources in polar regions, the ice covering of hull and all kinds of equipment of navigation ships brings serious safety risks to the safe navigation of polar ships. Thus, research of anti-icing coatings for polar ships and offshore equipment gradually becomes a hot research topic nowadays. Superhydrophobic coatings have excellent ice-resistance properties. However, its practical application is limited to some extent. This paper presents a review on the icing theory, the theoretical models of superhydrophobicicity, and the anti-icing properties of superhydrophobic interfaces. Then the application of superhydrophobic coatings with different preparation methods in the field of anti-icing is discussed and summarized. Finally, aiming at the shortcomings of superhydrophobic coating in deicing, the strategy of superhydrophobic coating with photothermal and electrothermal functions was proposed, and the current research status was comprehensively introduced.

Key words： anti-icing coating superhydrophobicity photothermal de-icing electrothermal de-icing polar region

收稿日期: 2023-02-24 32134.14.1005.4537.2023.046

ZTFLH:

TG178

基金资助:国家自然科学基金(41976039);上海市深远海洋装备材料工程技术中心基金(19DZ2253100)

通讯作者: 类延华，E-mail: yhlei@shmtu.edu.cn，研究方向为导电聚合物功能涂层、抗冰涂层的应用开发
刘涛，E-mail: liutao@shmtu.eud.cn，研究方向为防腐涂层设计开发、微生物腐蚀研究

Corresponding author: LEI Yanhua, E-mail: yhlei@shmtu.edu.cn
LIU Tao, E-mail: liutao@shmtu.eud.cn

作者简介: 姜伯晨，男，1993年生，博士，讲师

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图1 斜面上的接触角滞后和润湿理论模型

图2 均匀形核和非均匀形核的突破能垒对比示意图[30]

图3 水滴(初始直径D0 = 2 mm，冲击速度V0 =1 m·s-1)对超疏水表面的撞击过程示意图[39]

图4 在光滑、纳米结构和微纳米结构的金属表面上的冰形成过程光学图像[42]

表1 超疏水抗冰涂层的制备方法及各项性能表征总结

图5 光热材料光照生热过程原理

图6 ATP、PPY/ATP和PPY/ATP@十六烷基POS涂层和其在1个太阳光照下的表面温度随照射时间的变化，以及相应的ATP、PPY、PPY/ATP和PPY/ATP@十六烷基POS涂层在一定时间间隔内的红外图像[64]

Preparation method

Photothermal materials /

substrate

Delayed freezing time

Adhesion of ice

Photothermal performance

Citation

Heating temperature

under light

Ice melting time

under light

Other

performance

Laser etching and PFTS modification

Moth eye structure/Aluminum plate

1085 s vs 300 s

at -15^oC

The temperature rises to 80^oC in 300 s/ by 1 sun (0.1 W/cm²)

Melt the 10 mm ×

10 mm ice in 240 s

/by one sun

20 icing / deicing cycles, High durability and wear resistance

[65]

Electron beam vapor deposition

TiN,PTFE/Q234

78 s vs

20 s

at -10^oC

The temperature rises to 85^oC in 600 s/ by NIR irradiation,

808 nm, 0.1 mW/cm²

Melt the 25 mm ×

25 mm × 3 mm ice

in 50 s/ by NIR irradiation, 0.1 W/cm²

High temperature thermal stability, excellent corrosion resistance

[66]

Spraying method

SiC, SiO₂/

copper mesh

82 s vs

43 s

at -30^oC

1.66 kPa vs

5.87 kPa

The temperature rises to 48.3^oC in 60 s

/by NIR irradiation,

808 nm, 2.5 W/cm²

Melt the ice in

300 s/by NIR irradiation

(2.5 W/cm²)

High heat conversion efficiency, high flexibility and wear resistance

[67]

Spraying method

Melanin nanoparticles/glass

144 s vs

63 s

at -20^oC

25.65 kPa vs

104.13 kPa

The temperature rises to 68.5^oC in 600 s

/by 1 sun

(0.1 W/cm²)

Melt the 3 mm thick ice in 600 s/by one sun (0.1 W/cm²)

10 icing /

deicing cycles

[68]

Spraying method

FMWCNTs/Aluminum plate

364 s vs

23 s

at -10^oC

The temperature rises to 55.7^oC in 600 s

/by 1 sun (0.1 W/cm²)

Melt the 2 mm thick ice in 900 s/by one sun (0.1 W/cm²)

Photothermal self - healing performance, high heat conversion efficiency

[69]

Spraying method

SiO₂/SiC/

EVA Plate

152 s vs

29 s

at -30^oC

4.42 kPa vs

52.17 kPa

The temperature rises to 315^oC in 10 s /by NIR

(808 nm)

Melt the 25 mm ×

35 mm × 3 mm ice

in 180 s /by NIR

(808 nm)

5 icing /

deicing cycles

[70]

Spraying method

SiC/CNTs/

EVA Plate

66 s vs

15 s

at -30^oC

2.65 kPa

25.65 kPa

The temperature rises to 172.6^oC in 60 s /by NIR (808 nm)

Melt the 25 mm ×

45 mm × 30 mm ice in 250 s/by NIR

(808 nm)

high heat conversion efficiency

[71]

Spraying method

Fe₃O₄ /

glass

2878 s vs 50 s

at -15^oC

213.7 kPa vs

399.9 kPa

The temperature rises to 38^oC in 300 s

/by fluorescent lamp

(75 W)

Melt the ice in

232 s/by fluorescent lamp (75 W)

10 icing /

deicing cycles

[72]

表2 光热超疏水抗冰涂层的各项性能表征总结

图7 焦耳热传递示意过程

图8 FSGF-T200薄膜的电热除冰原理，在不同施加电压下的焦耳加热曲线和施加15 V直流电压后FSGF-T200的红外图像，除霜与除冰过程[86]

图9 涂层光生热、电生热、光电生热和磁生热作用过程

图10 PESC涂层在施加不同光强下的光照生热曲线，在施加不同电压下的焦耳生热曲线，在9.0 V电压下施加不同光强下的生热曲线，在同时施加不同电压和光强下的红外图像，在施加不同电压和光强下的水滴结冰过程和红外图[88]

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