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Journal of Chinese Society for Corrosion and protection  2015, Vol. 35 Issue (5): 379-385    DOI: 10.11902/1005.4537.2014.228
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Investigation Progress on Corrosion Behavior of Supercr-itical CO2 Transmission Pipelines Containing Impurities in CCS
Chong SUN1,Yong WANG1,Jianbo SUN1(),Tao JIANG1,Weimin ZHAO1,Yanchun ZHANG2
1. School of Mechanical & Electronic Engineering, China University of Petroleum, Qingdao 266580, China
2. China Petroleum LONGWAY Engineering Project Management Co. Ltd., Langfang 065000, China
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Abstract  

A range of impurities may exist in supercritical CO2 stream of transmission pipelines for carbon capture and storage (CCS) process, which are the potential corrosive factors to induce operational risks of the supercritical CO2 transmission pipeline. The impurities induced inner side corrosion of supercritical CO2 pipelines may become the bottleneck restricting the development and application of CCS. This paper reviews the recent research progress on the corrosion behavior of pipelines for supercritical CO2 transmission. The potential corrosion risks and the impact factors on corrosion are analyzed. The influence of impurities on the phase behavior, water chemistry characteristics, corrosion scales and the corrosion mechanism of transmission pipelines is also discussed. The shortcomings in the present investigations and the key scientific problems for further research are also pointed out.
Key words:  carbon capture and storage      supercritical CO2      impurity      corrosion scale      corrosion mechanism     
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Chong SUN
Yong WANG
Jianbo SUN
Tao JIANG
Weimin ZHAO
Yanchun ZHANG

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Chong SUN, Yong WANG, Jianbo SUN, Tao JIANG, Weimin ZHAO, Yanchun ZHANG. Investigation Progress on Corrosion Behavior of Supercr-itical CO2 Transmission Pipelines Containing Impurities in CCS. Journal of Chinese Society for Corrosion and protection, 2015, 35(5): 379-385.

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https://www.jcscp.org/EN/10.11902/1005.4537.2014.228     OR     https://www.jcscp.org/EN/Y2015/V35/I5/379

Ref. CO2 H2O O2 SOx NOx H2S CH4 N2 CO
DYNAMIS[6] ＞95.5 0.05 Aquifer＜4, EOR＜0.01~0.1 0.01 0.01 0.02 Aquifer＜4, EOR＜2 ＜4 0.2
Kinder Morgan[11] 95 0.063 0.001 --- --- 0.001~0.02 5 4 ---
Weyburn[11] 96 0.002 ＜0.007 --- --- 0.9 0.7 ＜0.03 0.1
Sheep Moutain[11] 96.8~97.4 0.0315 --- --- --- --- 1.7 0.6~0.9 ---
Central Basin[11] 98.5 0.063 ＜0.001 --- --- ＜0.002 0.2 1.3 ---
Literature data[12] 90~95 0.001~0.063 0.001~0.1 0.01~0.15 0.01~0.15 0.01~1.50 ＜5 ＜4 0.01~4
Table 1  Controlling of impurity content of supercritical CO2 in the process of CCS
Steel Temperature ℃ Pressure MPa Volume fraction of H2O / % Volume fraction of O2 / % Volume fraction of SO2 / % Volume fraction of NO2 / % Corrosion rate mma-1
X65[4] 50 4~8 Saturability 0 0 0 ~0.2
X70[14] 22 6.3 0.149 0 0 0 No
X70[14] 22 6.3 0.244 0 0 0 Slight
X65[15] 20 10 0.122 0 0 0 No
X65[16] 50 8 Saturability 0 0 0 0.38
X65[16] 50 8 Saturability 4 1 0 ＞7
1010[17] 45 7.58 0.244 0.01 0 0 2.3
1010[17] 45 7.58 0.244 0 0.01 0 4.6
1010[17] 45 7.58 0.244 0 0 0.01 11.6
X65[18] 50 8 0.159 4 1 0 3.7
X70[19] 50 10 Saturability 0.1 0.2~2 0 0.2~0.9
X65[20] 25 10 0.0488 0 0.01~0.0344 0.0096~0.0478 0.005~1.6
X70[21] 50 10 RH: 50~60% 0.1 2 0 ~0.1
Table 2  Relevant research results about CO2 transmission pipeline corrosion in recent years
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