热障涂层金属粘结层制备与研究进展

doi:10.11902/1005.4537.2024.267

中国腐蚀与防护学报

2025, Vol. 45

Issue (1): 20-32 CSTR: 32134.14.1005.4537.2024.267 DOI: 10.11902/1005.4537.2024.267

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热障涂层金属粘结层制备与研究进展

张晗, 刘轩溱, 黄爱辉, 赵晓峰, 陆杰(

)

上海交通大学材料科学与工程学院上海市先进高温材料及精密成型重点研究室上海 200240

Manufacturing and Research Progress in Metallic Bond Coats for Thermal Barrier Coatings

ZHANG Han, LIU Xuanzhen, HUANG Aihui, ZHAO Xiaofeng, LU Jie(

)

Shanghai Key Laboratory of Advanced High-Temperature Materials and Precision Forming, School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China

引用本文:

张晗, 刘轩溱, 黄爱辉, 赵晓峰, 陆杰. 热障涂层金属粘结层制备与研究进展[J]. 中国腐蚀与防护学报, 2025, 45(1): 20-32.
Han ZHANG, Xuanzhen LIU, Aihui HUANG, Xiaofeng ZHAO, Jie LU. Manufacturing and Research Progress in Metallic Bond Coats for Thermal Barrier Coatings[J]. Journal of Chinese Society for Corrosion and protection, 2025, 45(1): 20-32.

全文: PDF(14840 KB) HTML

摘要:

热障涂层是航空发动机和地面燃气轮机提升工作效率、延长服役寿命的关键技术和重要手段。粘结层作为热障涂层系统中的重要组成部分，一方面可缓解陶瓷层和高温合金基体间的热不匹配应力，提高热障涂层系统热稳定性；另一方面，高温下通过生长一层致密且连续的Al₂O₃层，保护合金基体免受氧化和腐蚀。因此，粘结层性能直接决定了热障涂层系统的服役寿命。本文系统总结了传统粘结层材料、制备方法及其优缺点等方面的研究进展，同时介绍了新型高熵合金粘结层体系，重点关注其成分设计、结构及抗氧化性能等方面的研究现状及不足。最后，对粘结层材料的研究方向进行了展望。

关键词 ：热障涂层, 金属粘结层, 高温氧化, NiAl, MCrAlY, 高熵合金

Abstract：

Thermal barrier coatings (TBCs) are widely used to protect the key components of areo- and land-based turbine engines, which is a key technology and an important means to improve engines efficiency and extend service life. The bond coat, as an important component of the TBC system, can relieve the thermal mismatch between the ceramic topcoat and the superalloy substrate, and improve the thermal stability of the thermal barrier coating system. On the other hand, it protects the superalloy substrate from oxidation and corrosion at high temperatures by forming a dense and continuous of Al₂O₃ layer. Therefore, the service life of the TBCs is predominantly dependent on the performance of bond coat. In this paper, the research progress on the conventional bond coat materials and preparation methods, as well as their advantages and disadvantages are introduced. The newly high-entropy alloy bond coat system is introduced with emphasis on the research progress of composition design, structure and oxidation resistance, as well as its deficiencies. Finally, the research trend of high entropy alloy bond coat materials is prospected.

Key words： thermal barrier coatings metallic bond coat high-temperature oxidation NiAl MCrAlY high-entropy alloy

收稿日期: 2024-08-25 32134.14.1005.4537.2024.267

ZTFLH:

TG174

基金资助:国家自然科学基金(52201082; 51971139)

通讯作者: 陆杰，E-mail：lu-jie@sjtu.edu.cn，研究方向为热障涂层

Corresponding author: LU Jie, E-mail: lu-jie@sjtu.edu.cn

作者简介: 张晗，女，1994年生，博士生

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图1 Ni-Al体系二元相图[18]，Ni-Pt-Al三元体系在1100/1150 ℃的等温相图[22]及其在1150 ℃氧化100 h后氧化膜组成[19]

图2 两种NiPtAl涂层的微观结构[16,23]

表1 工业燃气轮机和航空发动机中的商用MCrAlY产品[41] (mass fraction / %)

表2 MCrAlY涂层制备工艺的优缺点

图3 3种不同喷涂技术制备的典型MCrAlY涂层形貌[44,53]

图4 AlCoCrFeNi高熵合金纳米共格A2/B2相结构[67]

图5 AlCoCrFeNi和AlCoCr0.8FeNi高熵合金的相变和微观结构分析[70]

图6 AlCoCrFeNiY高熵合金粘结层TEM分析[79]

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