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中国腐蚀与防护学报  2025, Vol. 45 Issue (2): 283-295     CSTR: 32134.14.1005.4537.2024.260      DOI: 10.11902/1005.4537.2024.260
  临氢关键材料服役行为研究专刊 本期目录 | 过刊浏览 |
掺氢天然气管材及焊缝的氢损伤行为研究进展
白云龙1,2, 冷冰3, 韦博鑫1,2,4, 董立谨5, 于长坤1, 许进1,2, 孙成1,2()
1.中国科学院金属研究所 辽宁沈阳土壤大气环境材料腐蚀国家野外科学观测研究站 沈阳 110016
2.中国科学技术大学材料科学与工程学院 沈阳 110016
3.中国石油辽河油田公司采油工艺研究院 盘锦 110206
4.南洋理工大学机械与航空航天工程学院 新加坡 639798
5.西南石油大学新能源与材料学院 成都 610500
Research Progress on Hydrogen Damage Behavior of Pipeline Steel and Welds for Transportation of Hydrogen-blended Natural Gas
BAI Yunlong1,2, LENG Bing3, WEI Boxin1,2,4, DONG Lijin5, YU Changkun1, XU Jin1,2, SUN Cheng1,2()
1.Liaoning Shenyang Soil and Atmosphere Corrosion of Material National Observation and Research Station, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016, China
2.School of Materials Science and Engineering, University of Science and Technology of China, Shenyang 110016, China
3.Oil Production Technology Research Institute of China Petroleum Liaohe Oilfield Company, Panjin 110206, China
4.School of Mechanical and Aerospace Engineering, Nanyang Technological University, Singapore 639798, Republic of Singapore
5.School of New Energy and Material, Southwest Petroleum University, Chengdu 610500, China
引用本文:

白云龙, 冷冰, 韦博鑫, 董立谨, 于长坤, 许进, 孙成. 掺氢天然气管材及焊缝的氢损伤行为研究进展[J]. 中国腐蚀与防护学报, 2025, 45(2): 283-295.
Yunlong BAI, Bing LENG, Boxin WEI, Lijin DONG, Changkun YU, Jin XU, Cheng SUN. Research Progress on Hydrogen Damage Behavior of Pipeline Steel and Welds for Transportation of Hydrogen-blended Natural Gas[J]. Journal of Chinese Society for Corrosion and protection, 2025, 45(2): 283-295.

全文: PDF(19965 KB)   HTML
摘要: 

天然气管道掺氢输送是当前氢能输送最经济有效的方式之一。然而，掺氢管材在临氢环境中服役时，管线内部的氢原子会渗透到管材中。服役过程中的高压氢环境、应力和腐蚀介质等因素也会对管线造成损伤，严重威胁掺氢管线的服役安全。基于上述问题，本文概述了管材与氢的相容性问题，从管材及焊缝组织的氢渗透行为和研究方法入手，分析了氢在管材内的吸附和扩散问题，并从影响因素等方面综述了掺氢管材及焊接组织的氢损伤形式和机理。研究结果可为掺氢天然气管材的选择、设计及安全服役提供理论基础，促进氢能经济的安全发展。
关键词 ： 掺氢管线,  氢促失效,  氢渗透,  氢致开裂,  氢扩散    
Abstract：

To transfer the blend natural gas with hydrogen through the existing natural gas pipelines is currently one of the most economical and effective ways for hydrogen energy transportation. However, when pipelines in contact with hydrogen-enriched atmospheres, hydrogen atoms can permeate into the pipeline steels inducing hydrogen damages, which can severely threaten the safety of pipelines. Factors such as high-pressure, stress, and corrosive media during service may be involved to the damage of pipelines. Based on these issues, this paper summarizes the compatibility of pipeline steels with hydrogen, analyzes the adsorption and diffusion of hydrogen within the steels from the perspectives of hydrogen permeation behavior and testing methods. Additionally, it summarizes the forms and mechanisms of hydrogen damage in pipeline steels and welds of transportation of hydrogen-blended natural gas, in terms of the relevant influencing factors. The findings may provide a theoretical basis for the selection, design, and safe service of transporting hydrogen-blended natural gas pipelines, promoting the safe development of the hydrogen economy.
Key words： hydrogen blending pipelines    hydrogen-induced failure    hydrogen permeation    hydrogen induced cracking (HIC)    hydrogen diffusion
收稿日期: 2024-08-18      32134.14.1005.4537.2024.260
ZTFLH:  TG172  
基金资助:国家自然科学基金(52301115);国家自然科学基金(51871228);中国科院金属研究所创新基金(2023-PY12)
通讯作者: 孙成，E-mail：chengsun@imr.ac.cn，研究方向为管线钢环境服役损伤机制
Corresponding author: SUN Cheng, E-mail: chengsun@imr.ac.cn
作者简介: 白云龙，男，1990年生，博士生
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https://www.jcscp.org/CN/10.11902/1005.4537.2024.260      或      https://www.jcscp.org/CN/Y2025/V45/I2/283

图1  氢扩散系数与温度函数关系[24]
图2  未掺氢和掺氢环境下铁氧体悬臂梁的扫描电镜图像[25]
图3  氢分子扩散进入板条状贝氏体(LB)和粒状贝氏体(GB)的示意图[31]
图4  H2在Fe金属(110)面吸附解离过程的电子云密度分布变化等势面[33]
图5  氢原子从吸附到扩散进入γFe(111)表面势能变化过程[34]
图6  X80钢管氢浓度分布云图[35]
图7  施加300 MPa的拉伸应力和氢微印处理后试样的SEM图像[45]
图8  原始奥氏体晶界(PAGB)和板条界(LB)在不同氢通量条件下的氢扩散示意图[46]
图9  X80钢及HAZ各亚区的氢渗透曲线[36]
图10  X100管线钢HIC裂纹扩展形貌[48]
图11  氢化对螺位错弓出运动的影响[64]
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