海底管道<strong>CO<sub>2</sub></strong> 腐蚀特性及预测模型研究进展

doi:10.11902/1005.4537.2022.366

中国腐蚀与防护学报

2023, Vol. 43

Issue (6): 1225-1236 CSTR: 32134.14.1005.4537.2022.366 DOI: 10.11902/1005.4537.2022.366

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海底管道CO₂ 腐蚀特性及预测模型研究进展

朱烨森¹^,²(

), 蔡锟¹, 胡葆文¹, 夏云秋¹, 胡涛勇¹, 黄一²

^1.中国电建集团华东勘测设计研究院有限公司杭州 311122
^2.大连理工大学工业装备结构分析国家重点实验室大连 116024

Research Progress on Characteristics and Prediction Models of Carbon Dioxide Induced Corrosion for Submarine Pipelines

ZHU Yesen¹^,²(

), CAI Kun¹, HU Baowen¹, XIA Yunqiu¹, HU Taoyong¹, HUANG Yi²

^1.Power China Huadong Engineering Co., Ltd., Hangzhou 311122, China
^2.State Key Laboratory Analysis for Industrial Equipment, Dalian University of Technology, Dalian 116024, China

引用本文:

朱烨森, 蔡锟, 胡葆文, 夏云秋, 胡涛勇, 黄一. 海底管道CO₂ 腐蚀特性及预测模型研究进展[J]. 中国腐蚀与防护学报, 2023, 43(6): 1225-1236.
Yesen ZHU, Kun CAI, Baowen HU, Yunqiu XIA, Taoyong HU, Yi HUANG. Research Progress on Characteristics and Prediction Models of Carbon Dioxide Induced Corrosion for Submarine Pipelines[J]. Journal of Chinese Society for Corrosion and protection, 2023, 43(6): 1225-1236.

全文: PDF(3130 KB) HTML

摘要:

介绍了海底管道的CO₂腐蚀机理，具体涉及化学反应过程、电化学反应过程、传质过程和成膜过程。其次，总结了海底管道CO₂腐蚀影响因素，主要包括元素成分、显微组织决定的材料自身因素，以及介质成分、温度、pH等决定的外部环境因素。汇总了各影响因素对腐蚀速率的经验/半经验规律。重点归纳了海底管道CO₂腐蚀模型，详细介绍了原理模型法和经验模型法在腐蚀评估和预测中的控制步骤和边界条件。

关键词 ：海底管道, CO₂腐蚀, 腐蚀模型, 腐蚀预测, 腐蚀评估

Abstract：

Firstly, the mechanism of CO₂ induced corrosion of submarine pipeline is introduced, including chemical reaction process, electrochemical reaction process, mass transfer process and film formation process. Secondly, the influencing factors of CO₂ induced corrosion of submarine pipelines are summarized, which mainly include material factors determined by chemical composition and microstructure, and external environmental factors determined by medium composition, temperature and pH, etc. At the same time, the empirical/semi-empirical regulations of the corrosion rate versus influencing factors are summarized. Finally, the models of CO₂ induced corrosion of submarine pipeline is summarized, and the control steps and boundary conditions of the principle model and empirical model for corrosion-assessment and -prediction are introduced in detail.

Key words： submarine pipeline carbon dioxide corrosion corrosion model corrosion prediction corrosion assessment

收稿日期: 2022-11-23 32134.14.1005.4537.2022.366

ZTFLH:

TG174

基金资助:中国博士后科学基金(2022M722955);工业装备结构分析国家重点实验室开放课题基金(GZ22118)

通讯作者: 朱烨森，E-mail: zhuyesen@163.com，研究方向为海工/水工金属结构腐蚀监测及防腐

Corresponding author: ZHU Yesen, E-mail: zhuyesen@163.com

作者简介: 朱烨森，男，1992年生，博士生

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https://www.jcscp.org/CN/10.11902/1005.4537.2022.366 或 https://www.jcscp.org/CN/Y2023/V43/I6/1225

图1 CO2分压对腐蚀及成膜的影响[87]

图2 pH对腐蚀及成膜的影响[87]

图3 CO2腐蚀模型示意图

Process

$I 0, r e f$

A·m^-2

C r e f, H +

mol·L^-1

$C r e f, H 2 C O 3$

mol·L^-1

$Δ H$

kJ·mol^-1

$T r e f$

$b$

E_rev

Fe oxidation

37.5

293.15

2.3RT/1.5F

-0.488

H⁺ reduction

0.02

0.0001

293.15

2.3RT/0.5F

-0.24

H₂CO₃ reduction

0.014

0.0001

293.15

2.3RT/0.5F

-0.24

表1 交换电流密度计算参数[32,109]

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