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Journal of Chinese Society for Corrosion and protection  2021, Vol. 41 Issue (3): 277-288    DOI: 10.11902/1005.4537.2020.089
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Research Progress on Corrosion Resistance of Metallic Glasses
WANG Dongliang, DING Huaping, MA Yunfei, GONG Pan(), WANG Xinyun
State Key Laboratory of Material Processing and Die & Mould Technology, School of Material Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
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Abstract  

Because of their unique amorphous structure, metallic glasses (MGs) exhibit better corrosion resistance compared with traditional crystalline metals and alloys. Thus, MGs have broad application prospects as novel corrosion-resistant materials. The research progress of corrosion resistance of MGs was summarized. The influence factors, such as the alloy composition, microstructure, preparation method, corrosion environment, surface state, stress state etc. on the corrosion resistance of MGs were introduced. The routes to improve the corrosion resistance of MGs were proposed. Finally, the future development trends of corrosion resistance of MGs were discussed and prospected.
Key words:  metallic glass      corrosion resistance      influence factor      improving method     
Received:  24 May 2020     
ZTFLH:  TG174  
Fund: Natural Science Foundation of Hubei Provincial(2018CFB576);National Natural Science Foundation of China(51725504);Fundamental Research Funds for the Central Universities(2018KFYRCPT001)
Corresponding Authors:  GONG Pan     E-mail:  pangong@hust.edu.cn
About author:  GONG Pan, E-mail: pangong@hust.edu.cn
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Dongliang WANG
Huaping DING
Yunfei MA
Pan GONG
Xinyun WANG

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WANG Dongliang, DING Huaping, MA Yunfei, GONG Pan, WANG Xinyun. Research Progress on Corrosion Resistance of Metallic Glasses. Journal of Chinese Society for Corrosion and protection, 2021, 41(3): 277-288.

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https://www.jcscp.org/EN/10.11902/1005.4537.2020.089     OR     https://www.jcscp.org/EN/Y2021/V41/I3/277

Fig.1  Corrosion behavior in metallic glasses (MGs) and common stainless steels (SSs) in 3.5%NaCl solution (a), 1 mol/L HCl solution (b) and 1 mol/L NaOH solution (c)
ElementContent x(Atomic fraction / %)Base alloy (Atomic fraction / %)Corroding solutionEffect on corrosion resistanceReferences
Sr0~1%Mg66Zn30Ca4-xSrxPhosphate-buffered salineEnhanced[33]
1%~1.5%Deteriorated
Y0~2.5%(Zr58Nb3Cu16Ni13Al10)100-xYx0.5 mol/L H2SO4Deteriorated[30]
1%(Zr55Al10Cu30Ni5)99YxPhosphate-buffered salineEnhanced[20]
Nb0~20%Zr46Cu(30.14-x)NbxAg8.36Al8Be7.50.1 mol/L HClEnhanced[34]
0.5 mol/L NaClEnhanced
0.5 mol/L H2SO4Enhanced
Nd0~0.5%Mg68-xZn28Ca4NdxSimulated body fluidEnhanced[25]
0.5%~1.5%Deteriorated
Cr0~30%CrxFe56-xCo7Mo14C15B6Y21 mol/L HClEnhanced[32]
30%~45%No difference
0~29.4%CrxFe58.8-xMo14.7C14.7B9.8Y21 mol/L HClEnhanced[35]
29.4%~44.1%No difference
0~8.3%Fe71.4-xC7.1Si4.4B6.5P8.6CrxAl2.09.7 mol/L H2SO4Enhanced[22]
8.3%~12.3%Deteriorated
0~5%Fe79.5-xSi9.5B11Crx0.1 mol/L NaClEnhanced[36]
B0~5%Zr66.7-xNi33.3Bx0.5 mol/L NaClB0.3＞B0.1, B0.5＞B0[19]
1 mol/L HClB0.5＞B0.1, B0.3＞B0
2 mol/L NaOHB0.1＞B0.5＞B0.3, B0
Co0~4%(Zr46Cu46Al8)100-xCox3.5%NaClEnhanced[28]
Ti0~4%(Cu37.6Zr46Ag8.4Al8)100-xTix1 mol/L NaOHEnhanced[26]
1 mol/L H2SO4Enhanced
1 mol/L H2SO4+0.01 mol/L NaClEnhanced
1 mol/L H2SO4+0.1 mol/L NaClEnhanced
Ag0~9%Zr53Co23.5-xAl23.5AgxPhosphate-buffered salineEnhanced[29]
Si0~2%Fe85.2SixB9P5-xCu0.8Boric-borate buffer solutionEnhanced[37]
C0~3%Fe73.5Cu1Nb3Si13.5CxB99-x0.1 mol/L H2SO4Enhanced[38]
Mn0~1.5%(Mg65Zn30Ca5)100-xMnxSimulated body fluidDeteriorated[24]
Ce3%~7%Al93-xCo7Cex0.6 mol/L HClCe4 is the best[39]
Au0~3%Ca47Mg18Zn35-xAuxRinger's solutionEnhanced[40]
P0~15%Fe43Cr16Mo16(C, B, P)251, 6, 12 mol/L HClP＞B, C[21]
Ni0~0.4%[(Fe1-xNix)0.75B0.2Si0.05]96Nb40.5 mol/L HClEnhanced[27]
0.5 mol/L H2SO4Enhanced
0.5 mol/L NaOHEnhanced
Hf0~5%Zr55Ti3HfxCu32-xAl100.6 mol/L NaClEnhanced[31]
1 mol/L HClEnhanced
1 mol/L H2SO4Enhanced
Table 1  Summary of the effect of adding alloying elements on corrosion resistance
Fig.2  Potentiodynamic polarization curves of the as-cast and isothermally annealed Zr65Cu17.5Fe10Al7.5 bulk metallic glasses with different times in 3.5%NaCl solution[41]
Fig.3  FESEM images of corroded surface of the as-cast rod (5 mm) (a) and as-annealed rod (3 mm) (b) in the seawater solution[47]
Fig.4  Relationship between Ecorr and pH of Zr50.7Ni28Cu9Al12.3 bulk metallic glasses in 1 mol/L HCl, 0.5 mol/L H2SO4 and 0.5 mol/L NaCl solution[57]
Fig.5  Surface morphologies of carbon implanted (a) and untreated (b) Co-Cr-Mo alloy after corrosion tests[72]
Fig.6  Potentiodynamic polarization curves in 3.5%NaCl solution at room temperature for: (a) Fe71-xCrxMo3.5Ni5P10C4B4Si2.5 amorphous ribbons, (b) x=8 alloy (Fe69.88Cr8.26Mo6.67Ni5.83P6.15C0.95B0.86Si1.4), super duplex stainless steels UNSS32750 (Fe62.99Cr25.15Mo3.43Ni6.74P0.03C0.02Si0.55N0.27Mn0.69Cu0.13), austenitic steel AISI 316L (Fe65.16Cr17.54Mo2.47Ni12.3P0.02C0.03Si0.44Mn1.84), amorphous steel (Fe51.29Cr14.92Mo25.7C3.45B1.24Y3.4). The chemical compositions are given in mass percent for comparison[79]
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