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中国腐蚀与防护学报  2021, Vol. 41 Issue (6): 748-756    DOI: 10.11902/1005.4537.2020.167
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微生物腐蚀杀菌剂研究进展
何勇君1, 张天遂2, 王海涛3, 张斐2, 李广芳2, 刘宏芳2()
1.中国石化销售有限公司华南分公司 广州 510000
2.华中科技大学能量转换与存储材料化学教育部重点实验室 材料化学与服役实效湖北省重点实验室 化学与化工学院 武汉 430074
3.中国特种设备检测研究院 北京 100029
Research Progress of Biocides for Microbiologically Influenced Corrosion
HE Yongjun1, ZHANG Tiansui2, WANG Haitao3, ZHANG Fei2, LI Guangfang2, LIU Hongfang2()
1.SINOPEC Sales Co. Ltd. , (South China), Guangzhou 510000, China
2.Key Laboratory of Material Chemistry for Energy Conversion and Storage, Ministry of Education, Hubei Key Laboratory of Material Chemistry and Service Failure, School of Chemistry and Chemical Engineering, Huazhong University of Science and Technology, Wuhan 430074, China
3.China Special Equipment Inspection and Research Institute (CSEI), Beijing 100029, China
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摘要: 

结合近年来杀菌剂的研究和应用情况，针对不同类型微生物腐蚀现象，综述了油气田中用于防控细菌腐蚀的季铵盐类、胍类、杂环类和复配型杀菌剂的研究进展。对于目前研究较少的真菌和藻类所造成的微生物腐蚀，本文介绍了真菌和藻类诱导的金属腐蚀行为以及目前针对真菌和藻类杀菌剂的研究进展和应用情况。在此基础上总结了杀菌剂应用所面临的问题和未来发展趋势，为微生物腐蚀防护和杀菌剂的研究及合理使用提供参考。
关键词 ： 杀菌剂,  微生物腐蚀,  细菌,  真菌,  藻类    
Abstract：

Based on the research and application of biocides in recently years, the research progress of quaternary ammonium salts biocides, guanidine biocides, heterocyclic biocides and compounds biocides used in the prevention and control of microbiologically influenced corrosion (MIC) in oil and gas fields is reviewed. The MIC induced by fungus and algae as well as the research progress of corresponding biocides are introduced. On this basis, this article summarizes the application, challenges and future development trends of biocides, providing references for the research of microbial corrosion protection and rational use of biocides.
Key words： biocides    microbiologically influenced corrosion    bacteria    fungus    alga
收稿日期: 2020-09-23     
ZTFLH:  S482.2  
基金资助:国家重点研发计划(2017YFC0805000);中国石油化工股份有限公司项目(319008-8)
通讯作者: 刘宏芳     E-mail: liuhf@hust.edu.cn
Corresponding author: LIU Hongfang     E-mail: liuhf@hust.edu.cn
作者简介: 何勇君，男，1981年生，高级工程师
张天遂，男，1994年生，博士生
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引用本文:

何勇君, 张天遂, 王海涛, 张斐, 李广芳, 刘宏芳. 微生物腐蚀杀菌剂研究进展[J]. 中国腐蚀与防护学报, 2021, 41(6): 748-756.
Yongjun HE, Tiansui ZHANG, Haitao WANG, Fei ZHANG, Guangfang LI, Hongfang LIU. Research Progress of Biocides for Microbiologically Influenced Corrosion. Journal of Chinese Society for Corrosion and protection, 2021, 41(6): 748-756.

链接本文:

https://www.jcscp.org/CN/10.11902/1005.4537.2020.167      或      https://www.jcscp.org/CN/Y2021/V41/I6/748

图1  合成季铵盐聚乙烯亚胺纳米粒子[38,39]，表面修饰的二氧化硅纳米粒子[40]及溶胶-凝胶法制备的大分子单体[43]
图2  聚六亚甲基胍钼酸盐的合成[47]
Heterocyclic type of bactericidesCommorly used bactericidesUses and advantages
Ternary and quaternary heterocyclic compounds

Ethylene, Eopxiconazole,

Temocillin, Penicillin

Ternary heterocyclic compounds are often the key intermediates for the preparation of heterocyclic biocides. Temocillin and penicillin are beta amide heterocyclic fungicides with high fungicidal activity
Five-membered heterocyclic compounds

Thiazoles

Thiabendazole,

Etridiazole

Ethaboxam

Thiazole biocides possess a wide range of applications. In addition to inhibiting microbial corrosion, it can also be used to control harmful microorganisms in farmland

Furan

Fuberidazole, Fenfuram

Furalaxyl

Furan biocides have a wide range of biological activities, which can be used for sterilization, insecticidal and so on

Azole

Pyrrolnitrin, Fenpiclonil

Fludioxonil

Pyrrole biocides are derived from natural product nitropyrrolidins, among which imidazole methyl pyrrole compounds have the most prominent fungicidal activity

Oxazoles

Ibotenic acid, Hymexazol

Famoxadone, Glyodin

Imazalil, Oxpoconazole

Oxazoles biocides have good broad spectrum, bactericidal and permeability
Pyrazoles

Pyrazophos, Furametpyr

Pyraclostrobin

Pyrazole fungicide is a new type of heterocyclic biocides, which evolved from pyraclon

Triazoles[51]

Luotrimazole, Imazalil Bayleton[52]

Diniconazole, Triadimenol

Triazole biocides have excellent bactericidal properties and broad spectrum, and are the most widely used fungicides[51]
Six-member hetero-cyclic compoundsPyrimidines

Ferimzone, Mepanipyrim

Cyprodinil, Pyrimethanil

Pyrimidines are widely distributed and can be derived from a variety of natural extracts
PyridinesFiuazinam, Sodium pyrithione, FluopicofideThe research and application of six membered cyclic pyridine fungicides are few, they are potential fungicides
BenzimidazolesBenomyl, CarbendazimBenzimidazole biocides have the advantages of broad spectrum and low toxicity
表1  部分常规杂环杀菌剂
图3  模拟SPT在水溶液中Fe(110) 表面上的平衡吸附构型[53]
图4  碳钢在不同浓度BAC介质中浸泡5 d后表面小球藻生物膜的光学形貌[68]
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