Review on Research and Optimization of Corrosion Resistance of Thermal Sprayed Fe-based Amorphous Coatings

doi:10.11902/1005.4537.2022.138

Journal of Chinese Society for Corrosion and protection

2023, Vol. 43

Issue (2): 399-407 DOI: 10.11902/1005.4537.2022.138

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Review on Research and Optimization of Corrosion Resistance of Thermal Sprayed Fe-based Amorphous Coatings

ZHANG Ergeng, YANG Lei, YANG Hu, LIANG Dandan(

), CHEN Qiang(

), ZHOU Qiong, HUANG Biao

Shanghai Engineering Technology Research Center of Physical Vapor Deposition (PVD) Superhard Coatings and Equipment, Shanghai University of Technology, Shanghai 201418, China

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Abstract

Because of the advantages of high hardness and strength, superior thermal stability, good wear resistance, excellent corrosion resistance, outstanding soft magnetism, and low cost, Fe-based amorphous alloys exhibit a broad application prospect in many fields. However, the limited glass-forming ability and intrinsic plasticity greatly limit their application as engineering materials. Thereinto, Fe-based amorphous coatings prepared by thermal spraying technology can not only maintain their inherent characteristics but also avoid the aforementioned shortcomings, thus breaking through the limitation of engineering application. In this paper, the main preparation methods of Fe-based amorphous coatings by thermal spraying were comprehensively introduced, and the influencing factors of corrosion resistance, including the chemical composition, oxidation, pore, crystallization, and crack, were reviewed. Then, the methods to optimize the corrosion resistance of Fe-based amorphous coatings were summarized. Finally, the prospective research regarding the corrosion resistance of Fe-based amorphous coatings was proposed.

Key words: amorphous coating thermal spraying microstructure corrosion resistance

Received: 06 May 2022 32134.14.1005.4537.2022.138

ZTFLH:

TG174

Fund: National Natural Science Foundation of China(51901138);National Natural Science Foundation of China(51971148);Program of Shanghai Technology Research Leader(22XD1434500);Research Fund for Talents Introduction(YJ2022-31);Shanghai Natural Science Foundation of China(20ZR1455700)

About author: CHEN Qiang, E-mail: john_chen0826@163.com
LIANG Dandan, E-mail: liang.d.d@163.com

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Cite this article:

ZHANG Ergeng, YANG Lei, YANG Hu, LIANG Dandan, CHEN Qiang, ZHOU Qiong, HUANG Biao. Review on Research and Optimization of Corrosion Resistance of Thermal Sprayed Fe-based Amorphous Coatings. Journal of Chinese Society for Corrosion and protection, 2023, 43(2): 399-407.

URL:

https://www.jcscp.org/EN/10.11902/1005.4537.2022.138 OR https://www.jcscp.org/EN/Y2023/V43/I2/399

Table 1 Process characteristics of three common thermal spraying methods^[17,18]

Fig.1 Cross-sectional SEM image of arc-sprayed Fe-based amorphous coatings

Fig.2 Backscattered electron SEM image of the cross-sectional coating^[23]

Fig.3 Schematic diagram of corrosion process of Fe base coatings: (a) obstructed mass transport process; (b) electrolyte diffusion oxide layer; (c) induce local corrosion; (d) localized corrosion to the substrate^[35]

Fig.4 SEM morphologies (a, c) and the corresponding distribution maps of O (b, d) of the initial (a, b) and relaxed (c, d) amorphous coatings after corrosion^[36]

Fig.5 Corroded surface morphology (a) and the corresponding EDS mapping of O (b), Fe (c) and Cr (d) of Fe-based amorphous coating after the potentiodynamic polarization tests^[45]

Fig.6 Wettability angles of Fe-based amorphous coatings: (a) initial state and (b) relaxed state. The upper left is the AFM morphology of the corresponding sample^[36]

Fig.7 Schematic diagram of solution treatment of Fe-based amorphous coating: (a) schematic diagram of defects; (b) onset of corrosion; (c) selective dissolution; (d) hole sealing treatment^[54]

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