Characteristics on Electrochemical Noise of Pitting Corrosion for High Nitrogen Austenitic Stainless Steels

doi:10.11902/1005.4537.2016.242

Journal of Chinese Society for Corrosion and protection

2018, Vol. 38

Issue (1): 26-32 DOI: 10.11902/1005.4537.2016.242

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Characteristics on Electrochemical Noise of Pitting Corrosion for High Nitrogen Austenitic Stainless Steels

Pengliang AN¹, Ping LIANG¹(

), Jianmin REN¹, Yanhua SHI¹, Feng LIU¹, Siyao CHEN²

1 School of Mechanical Engineering, Liaoning Shihua University, Fushun 113001, China
2 North Hua Jin Chemical Industries Group Corporation, Panjin 124021, China

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Abstract

The pitting corrosion behavior of high nitrogen stainless steel (HNSS) and 316L stainless steel (316L SS) in 6%(mass fraction) FeCl₃ solution was compared by time domain, frequency domain spectrum and Weibull distribution analysis of electrochemical noise (EN) data. The time domain analysis results show that after immersion in the solution of 6%FeCl₃ for 5 h, the noise transient peaks appear on the measured potential noise and current noise of 316L SS, implying the occurrence of metastable pitting, however, at the same time, the noise transient peak does not appear on the EN plot of HNSS, while the potential noise and current noise only presented a slight high-frequency fluctuations, indicating the surface passivation film suffered from slightly attack, while presented ability of repassivation to certain extent. Moreover, the noise resistance fluctuation amplitude of 316L SS is larger than that of HNSS, which suggesting the ability in self-passivation and re-healing of the passivation film of HNSS is better than that of 316L SS. Plots of power spectral density show that the values of slope of high frequency and plateau intensity of white noise of 316L SS are larger than those of HNSS, and the relevant Weibull distribution analysis reveals that the rate of pitting inoculation for 316L SS is twice of that for HNSS, which predicating that the 316L SS is much prone to pitting than HNSS.

Key words: high nitrogen stainless steel electrochemical noise power spectral density

Received: 22 December 2016

ZTFLH:

TG174.3

Fund: Supported by National Natural Science Foundation of China (51175240)

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	Pengliang AN
	Ping LIANG
	Jianmin REN
	Yanhua SHI
	Feng LIU
	Siyao CHEN

Cite this article:

Pengliang AN, Ping LIANG, Jianmin REN, Yanhua SHI, Feng LIU, Siyao CHEN. Characteristics on Electrochemical Noise of Pitting Corrosion for High Nitrogen Austenitic Stainless Steels. Journal of Chinese Society for Corrosion and protection, 2018, 38(1): 26-32.

URL:

https://www.jcscp.org/EN/10.11902/1005.4537.2016.242 OR https://www.jcscp.org/EN/Y2018/V38/I1/26

Fig.1 Electrochemical noise signals of HNSS (a) and 316L SS (b) immersed in 6%FeCl₃ solution for 0 h

Fig.2 Electrochemical noise signals of HNSS (a) and 316L SS (b) after immersion in 6%FeCl₃ solution for 5 h

Fig.3 Electrochemical noise signals of HNSS (a) and 316L SS (b) after immersion in 6%FeCl₃ solution for 48 h

Fig.4 1/R_n vs time plots of HNSS and 316L SS in 6%FeCl₃ solution

Fig.5 PSD plots of HNSS and 316L SS after immersion in 6%FeCl₃ solution for 0 h (a), 48 h (b), 100 h (c) and 168 h (d)

Table 1 PSD parameters of HNSS and 316L SS

Fig.6 Cumulative probability plots of corrosion events for HNSS and 316L SS

Fig.7 Weibull plots of shot noises for HNSS and 316L SS

Table 2 Weibull function parameters of shot noises forHNSS and 316L SS

Fig.8 Variatios of pitting corrosion rate of HNSS and 316L SS with time

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